论文标题

通过局部层加热,在氧硝基硅薄膜中进行光学增强的第二次谐波生成

Optically enhanced second harmonic generation in silicon oxynitride thin films via local layer heating

论文作者

Lukeš, Jakub, Kanclíř, Vít, Václavík, Jan, Melich, Radek, Fuchs, Ulrike, Žídek, Karel

论文摘要

氮化硅中的第二个谐波生成(SHG)已在其他si3n4波导中的激光诱导的SHG增强方面进行了广泛的研究。这种增强已被归因于相干光藻效应引起的全光极。然而,尚未报道Si3n4薄膜的类似过程。我们的文章报道了在SI3N4薄膜中观察激光诱导的3倍SHG增强。观察到的增强功能具有许多类似于全光的特征,例如高度非线性功率依赖性,累积效应或与SI3N4-SI接口的连接。然而,低氧硅氧硝基薄膜的相同实验导致了复杂的行为,包括激光诱导的SHG还原。通过一项彻底的实验研究,观察到的结果归因于由多光子吸收引起的热诱导的SHG变化。这种行为表明,Sioxny-Si结构中光学诱导的SHG增强的起源可能是各种现象的复杂相互作用。

Strong second harmonic generation (SHG) in silicon nitride has been extensively studied-among others, in terms of laser-induced SHG enhancement in Si3N4 waveguides. This enhancement has been ascribed to the all-optical poling induced by the coherent photogalvanic effect. Yet, an analogous process for Si3N4 thin films has not been reported. Our article reports on the observation of laser-induced 3-fold SHG enhancement in Si3N4 thin films. The observed enhancement has many features similar to all-optical poling, such as highly nonlinear power dependence, cumulative effect, or connection to the Si3N4-Si interface. However, identical experiments for low-oxygen silicon oxynitride thin films lead to complex behavior, including laser-induced SHG reduction. By a thorough experimental study, the observed results were ascribed to heat-induced SHG variation caused by multiphoton absorption. Such behavior indicates that the origin of optically-induced SHG enhancement in SiOxNy-Si structures can be a complex interplay of various phenomena.

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