论文标题

建模散装晶体和薄膜中聚焦光束的非线性光学相互作用:一种现象学方法

Modeling nonlinear optical interactions of focused beams in bulk crystals and thin films: A phenomenological approach

论文作者

Spychala, Kai J., Amber, Zeeshan H., Eng, Lukas M., Rüsing, Michael

论文摘要

连贯的非线性光学微光谱镜是现代材料科学中常用的工具,因为它对许多不同的局部可观测物敏感,这些可观察物包括晶体对称性和振动特性。然而,信息的丰富性可能会带来数据解释的挑战,因为必须解散许多不同的效果,例如多种反射,界面上的相位跳跃或吉尼相的影响。为了促进解释,此处介绍的工作提出了易于使用的半分析建模ANSATZ,该建模基于使用高斯梁的已知分析解决方案。具体而言,我们将此Ansatz应用于(薄膜)光学材料的非线性光学响应。我们试图保存直观参数的含义,例如小相关和非线性相干相互作用长度。特别是,相干长度的概念扩展了,这是使用焦距时必须的。该模型随后应用于第二次谐波和第三谐波产生的示例性病例。我们观察到与实验数据和此外,尽管分析ANSATZ的限制和限制,但我们的模型在使用更严格的模拟时的性能类似。但是,它在计算能力方面的表现优于后者,需要超过三个订单的计算时间和较少的性能计算机系统。

Coherent nonlinear optical micro-spectroscopy is a frequently used tool in modern material science, as it is sensitive to many different local observables, which comprise, among others, crystal symmetry and vibrational properties. The richness in information, however, may come with challenges in data interpretation, as one has to disentangle the many different effects like multiple reflections, phase jumps at interfaces, or the influence of the Guoy-phase. In order to facilitate interpretation, the work presented here proposes an easy-to-use semi-analytical modeling ansatz, that bases upon known analytical solutions using Gaussian beams. Specifically, we apply this ansatz to compute nonlinear optical responses of (thin film) optical materials. We try to conserve the meaning of intuitive parameters like the Gouy-phase and the nonlinear coherent interaction length. In particular, the concept of coherence length is extended, which is a must when using focal beams. The model is subsequently applied to exemplary cases of second-harmonic and third-harmonic generation. We observe a very good agreement with experimental data and furthermore, despite the constraints and limits of the analytical ansatz, our model performs similarly well as when using more rigorous simulations. However, it outperforms the latter in terms of computational power, requiring more than three orders less computational time and less performant computer systems.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源