论文标题

基于钒的Kagome Metal SCV $ _6 $ SN $ _6 $中结构相变的光谱和带结构计算

Optical spectroscopy and band structure calculations of structural phase transition in the Vanadium-based kagome metal ScV$_6$Sn$_6$

论文作者

Hu, Tianchen, Pi, Hanqi, Xu, Shuxiang, Yue, Li, Wu, Qiong, Liu, Qiaomei, Zhang, Sijie, Li, Rongsheng, Zhou, Xinyu, Yuan, Jiayu, Wu, Dong, Dong, Tao, Weng, Hongming, Wang, Nanlin

论文摘要

在冷凝物理物理学中,具有kagome晶格的材料显示出一系列外来量子状态,包括电荷密度波(CDW),超导性和磁性。最近,发现金属间的金属SCV6SN6在92 k左右的root3xroot3x3 cdw中进行一阶结构相变。在这里,我们进行了一项光谱研究,并在整个结构过渡过程中结合了带结构的计算。我们的发现表明,由于结构过渡而没有任何可观察到的间隙形成行为,光反射率/电导率光谱的突然变化。光学测量和带计算实际上揭示了过渡后带结构的突然变化。重要的是要注意,这种相变是一阶类型的,它将其与常规密度波型冷凝区分开。我们的结果提供了对这个新独特的Kagome晶格中结构相变的起源的见解。

In condensed matter physics, materials with kagome lattice display a range of exotic quantum states, including charge density wave (CDW), superconductivity and magnetism. Recently, the intermetallic kagome metal ScV6Sn6 was discovered to undergo a first-order structural phase transition with the formation of a root3xroot3x3 CDW at around 92 K. The bulk electronic band properties are crucial to understanding the origin of the structural phase transition. Here, we conducted an optical spectroscopy study in combination with band structure calculations across the structural transition. Our findings showed abrupt changes in the optical reflectivity/conductivity spectra as a result of the structural transition, without any observable gap formation behavior. The optical measurements and band calculations actually reveal a sudden change of the band structure after transition. It is important to note that this phase transition is of the first-order type, which distinguishes it from conventional density-wave type condensations. Our results provide an insight into the origin of the structural phase transition in this new and unique kagome lattice.

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