论文标题
高Q纳米素化学在六角形硼硼元面启用的完整可见光谱上
High-Q nanophotonics over the full visible spectrum enabled by hexagonal boron nitride metasurfaces
论文作者
论文摘要
到目前为止,由于缺乏在完整的可见频谱上同时缺乏无损和高折射率(RI)材料,具有高质量(Q)因素的全dielectric光学元信息受到了阻碍。为了获得广泛的光谱覆盖率,由于带隙能量(因此是光损耗)和RI之间的反相关性,因此低索引材料的使用实际上是不可避免的。但是,对于MIE共振光子学,较小的RI与Q因子减少和模式体积限制有关。在这项工作中,我们利用连续体(BICS)中的对称性破裂状态有效抑制来自低索引(n〜2)范德华材料材料二氮化物(HBN)的辐射损失,从而在完整的可见光谱上实现了具有高Q的元脉冲。特别是,我们分析了低RI材料和高RI材料作为谐振组件的合理使用,并利用我们的见解以实验证明了Q因子以上300以上的Q因子尖锐的BIC共振,从单个HBN薄片中跨越了400 nm至1000 nm的波长。此外,我们利用增强的电力近场来展示第二次谐波生成(SHG),增强因子以上是102。我们的结果为实施低RI材料作为元词的光子介质提供了一个理论和实验框架。
All-dielectric optical metasurfaces with high quality (Q) factors have so far been hampered by the lack of simultaneously lossless and high refractive index (RI) materials over the full visible spectrum. To achieve broad spectral coverage, the use of low-index materials is, in fact, unavoidable due to the inverse correlation between the band-gap energy (and therefore the optical losses) and the RI. However, for Mie resonant photonics, smaller RIs are associated with reduced Q factors and mode volume confinement. In this work, we leverage symmetry-broken bound states in the continuum (BICs) to efficiently suppress radiation losses from the low-index (n~2) van der Waals material hexagonal boron nitride (hBN), realizing metasurfaces with high-Q resonances over the complete visible spectrum. In particular, we analyze the rational use of low and high RI materials as resonator components and harness our insights to experimentally demonstrate sharp BIC resonances with Q factors above 300, spanning wavelengths between 400 nm and 1000 nm from a single hBN flake. Moreover, we utilize the enhanced electric near-fields to demonstrate second harmonic generation (SHG) with enhancement factors above 102. Our results provide a theoretical and experimental framework for the implementation of low RI materials as photonic media for metaoptics.