论文标题

spin-1蜂窝状晶格kniaso $ _4 $中的Zig-Zag磁性和潜在的Kitaev相互作用

Zig-Zag magnetic order and potential Kitaev interactions in the spin-1 honeycomb lattice KNiAsO$_4$

论文作者

Taddei, K. M., Garlea, V. O., Samarakoon, A. M., Sanjeewa, L. D., Xing, J., Heitmann, T. W., Cruz, C. dela, Sefat, A. S., Parker, D.

论文摘要

尽管Kitaev Spin-Hamiltonian对发现并证实了量子旋转液态的含义令人难以置信。最近,通过开发Spin-1 Kitaev相互作用的显微镜​​描述,该模型的适用性已扩展。在这里,我们探索了一个候选Spin-1蜂窝系统Kniaso $ _4 $,该系统符合许多提出的标准以产生这种互动。批量测量结果显示出$ \ sim $ 19 K的抗铁磁过渡,通常对应用磁场很健壮。中子衍射测量测量显示了$ \ textbf {k} =(\ frac {3} {2} {2},0,0)$订购向量,这导致了众所周知的````Zigzag)''ZIG-ZAG“磁性结构”,这些磁性结构被认为是与旋转的基础状态相邻的。在实地差异的情况下,该阶段可以表现出强大的阶段,同时又表现出了阶段的序列,该方向是在实地方向上的方向,该方向是在现场上的方向,该方向是在现场上的方向,该方向是在现场上的指示。实验显示出明确的自旋波谱,没有证据表明旋转波的分数激发的连续性表明,扩展的Kitaev Spin-Hamiltonians对于Spectra建模是必需的,以便对光谱进行建模并重现ni unteration ni sumernation ni sublate insurtion ni sublate insultion ni sublate contription。将kniaso $ _4 $ $ _4 $靠近旋转的基态。

Despite the exciting implications of the Kitaev spin-Hamiltonian, finding and confirming the quantum spin liquid state has proven incredibly difficult. Recently the applicability of the model has been expanded through the development of a microscopic description of a spin-1 Kitaev interaction. Here we explore a candidate spin-1 honeycomb system, KNiAsO$_4$ , which meets many of the proposed criteria to generate such an interaction. Bulk measurements reveal an antiferromagnetic transition at $\sim$ 19 K which is generally robust to applied magnetic fields. Neutron diffraction measurements show magnetic order with a $\textbf{k}=(\frac{3}{2},0,0)$ ordering vector which results in the well-known ``zig-zag" magnetic structure thought to be adjacent to the spin-liquid ground state. Field dependent diffraction shows that while the structure is robust, the field can tune the direction of the ordered moment. Inelastic neutron scattering experiments show a well defined gapped spin-wave spectrum with no evidence of the continuum expected for fractionalized excitations. Modeling of the spin waves shows that the extended Kitaev spin-Hamiltonians is generally necessary to model the spectra and reproduce the observed magnetic order. First principles calculations suggest that the substitution of Pd on the Ni sublattice may strengthen the Kitaev interactions while simultaneously weakening the exchange interactions thus pushing KNiAsO$_4$ closer to the spin-liquid ground state.

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