论文标题

脉冲激光沉积的高质量$ MN_3SN $薄膜的外延生长

Epitaxial growth of high quality $Mn_3Sn$ thin films by pulsed laser deposition

论文作者

Gao, Dong, Peng, Zheng, Zhang, Ningbin, Xie, Yunfei, Yang, Yucong, Yang, Weihao, Xia, Shuang, Yan, Wei, Deng, Longjiang, Liu, Tao, Qin, Jun, Zhong, Xiaoyan, Bi, Lei

论文摘要

非电视抗抗铁磁铁WEYL半准$ MN_3SN $最近引起了极大的研究兴趣。尽管在$ MN_3SN $中观察到了较大的异常霍尔效应,异常的Nernst效果和磁光效应,但大多数研究都是基于单晶的。到目前为止,种植具有运输和光学特性的高质量外延$ MN_3SN $薄膜仍然具有挑战性。在这里,我们报告了由脉冲激光沉积(PLD)制造的外延$ MN_3SN $薄膜的结构,光学和传输特性。高度定向的$ Mn_ {3+X} sn_ {1-x} $(0001)和(11 $ \ bar2 $ 0)的外延膜在单晶$ al_2o_3 $和mgo substrates上成功增长。大型异常大厅效应(AHE)最多$ \ left | ΔR_H\ right | $ = 3.02 $μω\ CDOT CM $,以及纵向磁光kerr效应(LMOKE),其$θ_K$ = 38.1 mdeg在633 nm波长下在300 K温度下测量,可与$ MN_3SN $ $单晶相媲美。我们的工作表明,可以通过PLD制造高质量的$ MN_3SN $外延薄膜,为将来的设备应用铺平了道路。

Non-collinear antiferromagnet Weyl semimetal $Mn_3Sn$ have attracted great research interest recently. Although large anomalous Hall effect, anomalous Nernst effect and magneto-optical effect have been observed in $Mn_3Sn$, most studies are based on single crystals. So far, it is still challenging to grow high quality epitaxial $Mn_3Sn$ thin films with transport and optical properties comparable to their single crystal counterparts. Here, we report the structure, magneto-optical and transport properties of epitaxial $Mn_3Sn$ thin films fabricated by pulsed laser deposition (PLD). Highly oriented $Mn_{3+x}Sn_{1-x}$ (0001) and (11$\bar2$0) epitaxial films are successfully growth on single crystalline $Al_2O_3$ and MgO substrates. Large anomalous Hall effect (AHE) up to $\left| ΔR_H\right|$=3.02 $μΩ\cdot cm$, and longitudinal magneto-optical Kerr effect (LMOKE) with $θ_K$ = 38.1 mdeg at 633 nm wavelength are measured at 300 K temperature, which are comparable to $Mn_3Sn$ single crystals. Our work demonstrates that high quality $Mn_3Sn$ epitaxial thin films can be fabricated by PLD, paving the way for future device applications.

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