论文标题
激光直接编写六角硼硝化硼的可见旋转缺陷,用于基于旋转的技术的应用
Laser Direct Writing of Visible Spin Defects in Hexagonal Boron Nitride for Applications in Spin-Based Technologies
论文作者
论文摘要
在二维六边形氮化硼(HBN)中,具有光学地址的旋转引起了广泛的关注,因为它们在芯片量子设备(例如量子传感器和量子网络)中的潜在优势。在HBN中已经发现了各种自旋缺陷,但是除了带负电荷的硼($ v_b^ - $)外,尚无其他方便和确定性的生成方法。在这里,我们报告说,通过使用飞秒激光直接写作技术,我们可以在纳米级HBN薄片上确定性地创建光谱范围从550 nm到800 nm的旋转缺陷集合。在垂直于基板的磁场存在下检测到阳性的单峰光学检测到的磁共振(ODMR)信号,并且对比度可以达到0.8%。借助HBN薄片,底物和飞秒激光脉冲能的适当厚度,我们可以确定性地产生明亮的自旋缺陷阵列。我们的结果提供了一种方便的确定性方法,可以在HBN中创建自旋缺陷,这将激发更多的努力,以实现未来的研究和基于旋转技术(例如量子磁力计阵列)的应用。
Optically addressable spins in two-dimensional hexagonal boron nitride (hBN) attract widespread attention for their potential advantage in on-chip quantum devices, such as quantum sensors and quantum network. A variety of spin defects have been found in hBN, but no convenient and deterministic generation methods have been reported for other defects except negatively charged boron vacancy ($V_B^-$). Here we report that by using femtosecond laser direct writing technology, we can deterministically create spin defect ensembles with spectra range from 550 nm to 800 nm on nanoscale hBN flakes. Positive single-peak optically detected magnetic resonance (ODMR) signals are detected in the presence of magnetic field perpendicular to the substrate, and the contrast can reach 0.8%. With the appropriate thickness of hBN flakes, substrate and femtosecond laser pulse energy, we can deterministically and efficiently generate bright spin defect array. Our results provide a convenient deterministic method to create spin defects in hBN, which will motivate more endeavors for future researches and applications of spin-based technologies such as quantum magnetometer array.