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Data augmentation has been rare in the cyber security domain due to technical difficulties in altering data in a manner that is semantically consistent with the original data. This shortfall is particularly onerous given the unique difficulty of acquiring benign and malicious training data that runs into copyright restrictions, and that institutions like banks and governments receive targeted malware that will never exist in large quantities. We present MARVOLO, a binary mutator that programmatically grows malware (and benign) datasets in a manner that boosts the accuracy of ML-driven malware detectors. MARVOLO employs semantics-preserving code transformations that mimic the alterations that malware authors and defensive benign developers routinely make in practice , allowing us to generate meaningful augmented data. Crucially, semantics-preserving transformations also enable MARVOLO to safely propagate labels from original to newly-generated data samples without mandating expensive reverse engineering of binaries. Further, MARVOLO embeds several key optimizations that keep costs low for practitioners by maximizing the density of diverse data samples generated within a given time (or resource) budget. Experiments using wide-ranging commercial malware datasets and a recent ML-driven malware detector show that MARVOLO boosts accuracies by up to 5%, while operating on only a small fraction (15%) of the potential input binaries.