论文标题

钙钛矿量子点拓扑激光器

Perovskite quantum dot topological laser

论文作者

Tian, Jingyi, Tan, Qi Ying, Wang, Yutao, Yang, Yihao, Yuan, Guanghui, Adamo, Giorgio, Soci, Cesare

论文摘要

最近,各种拓扑激光概念实现了不受结构变形并耐受制造缺陷的稳健发光设备的演示。当前对具有拓扑边界的光子腔的实现通常受到远程耦合问题或方向性差的限制,并且需要进行复杂的设计和制造,以阻碍在小波长下运行。在这里,我们提出了一个基于两个具有独特Zak相的一维光子晶体之间的界面状态的拓扑腔设计,并展示了无光刻的单模钙钛矿激光器在绿色中排放。很少有溶液处理的全有机洞穴铅卤化物钙钛矿量子点用作超薄增益培养基。拓扑激光器具有平面设计,具有较大的输出光圈,类似于垂直腔表面发射激光器(VCSEL),并且可与增益培养基厚度的变化(从深度亚波长到厚的量子点膜)的变化。这种实验性观察也揭示了VCSEL的拓扑性质,通常在传统的Fabry-Perrot腔激光器的描述中被忽略。设计简单性和拓扑特性使该钙钛矿量子点激光体系结构适用于在可见光谱区域运行的低成本和制造耐受性垂直发射激光器。

Various topological laser concepts have recently enabled the demonstration of robust light-emitting devices that are immune to structural deformations and tolerant to fabrication imperfections. Current realizations of photonic cavities with topological boundaries are often limited by outcoupling issues or poor directionality and require complex design and fabrication that hinder operation at small wavelengths. Here we propose a topological cavity design based on interface states between two one-dimensional photonic crystals with distinct Zak phases and demonstrate a lithography-free, single-mode perovskite laser emitting in the green. Few monolayers of solution processed all-inorganic cesium lead halide perovskite quantum dots are used as ultrathin gain medium. The topological laser has planar design with large output aperture, akin to vertical-cavity surface-emitting lasers (VCSELs) and is robust against variations of the thickness of the gain medium, from deeply subwavelength to thick quantum dot films. This experimental observation also unveils the topological nature of VCSELs, that is usually overlooked in the description of conventional Fabry-Perot cavity lasers. The design simplicity and topological characteristics make this perovskite quantum dot laser architecture suitable for low-cost and fabrication tolerant vertical emitting lasers operating across the visible spectral region.

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