论文标题

Xuv h $ _2 $分子研究的XUV电离

XUV ionization of the H$_2$ molecule studied with attosecond angular streaking

论文作者

Serov, Vladislav V., Kheifets, Anatoli S.

论文摘要

我们研究h $ _2 $分子的attosentime photoionization的方向和两中性干扰效应。 h $ _2 $的XUV电离的时间分辨率是通过kheifets {\ em et al} [arXiv:2202.06147(2022)的阶段检索能力而获得的。一旦应用于h $ _2 $,该技术就会提供各向异性相和时间延迟,这两者都敏感地取决于分子轴方向。此外,光电子动量分布显示出非常清晰的两中心干扰模式。当由于Walter和Briggs引起的干扰公式时[J。物理。应用B {\ bf 32} 2487(1999)],有效的光电子动量似乎大于检测器的渐近动量。这种效果由光发射中心周围的分子电位孔解释。

We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular streaking demonstrated earlier by Kheifets {\em et al} [arXiv:2202.06147 (2022)]. Once applied to H$_2$, this technique delivers an anisotropic phase and time delay which both depend sensitively on the molecular axis orientation. In addition, the photoelectron momentum distribution displays a very clear two-center interference pattern. When the interference formula due to Walter and Briggs [J. Phys. B {\bf 32} 2487 (1999)] is applied, an effective photoelectron momentum appears to be greater than the asymptotic momentum at the detector. This effect is explained by a molecular potential well surrounding the photoemission center.

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