论文标题
来自融合多模式电子显微镜的成像原子尺度化学
Imaging Atomic-Scale Chemistry from Fused Multi-Modal Electron Microscopy
论文作者
论文摘要
使用电子显微镜以最小的噪声绘制低剂量的原子级化学的努力在根本上受到非弹性相互作用的限制。在这里,融合的多模式电子显微镜通过耦合在弹性散射(高角度环形暗场(HAADF))和弹性光谱信号(Eledon(Eledon)能量损失(eels)中编码的相关信息(eels)或原子能信号(ELON EDERON EDERS)或EDISEXIVE(EELSX),融合了纳米和原子分辨率的材料化学恢复高信噪比(SNR)。通过将这些同时获得的信号或方式链接,可以通过现有检测器硬件以明显较低的剂量成像纳米材料内的化学分布。在许多情况下,剂量要求可以减少一个数量级。对于异质纳米材料的模拟和实验原子分辨率数据,对化学的高SNR回收率进行了测试。
Efforts to map atomic-scale chemistry at low doses with minimal noise using electron microscopes are fundamentally limited by inelastic interactions. Here, fused multi-modal electron microscopy offers high signal-to-noise ratio (SNR) recovery of material chemistry at nano- and atomic- resolution by coupling correlated information encoded within both elastic scattering (high-angle annular dark field (HAADF)) and inelastic spectroscopic signals (electron energy loss (EELS) or energy-dispersive x-ray (EDX)). By linking these simultaneously acquired signals, or modalities, the chemical distribution within nanomaterials can be imaged at significantly lower doses with existing detector hardware. In many cases, the dose requirements can be reduced by over one order of magnitude. This high SNR recovery of chemistry is tested against simulated and experimental atomic resolution data of heterogeneous nanomaterials.