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In this paper, we investigate AdS/BCFT for curvature-squared gravity. To warm up, we start with Gauss-Bonnet gravity. We derive the one point function of stress tensor and show that the central charge related to the norm of displacement operator is positive for the couplings obeying causality constraints. Furthermore, by imposing the null energy condition on the end-of-the-world brane, we prove the holographic g-theorem for Gauss-Bonnet gravity. This corrects a wrong point of view in the literature, which claims that the holographic g-theorem is violated for Gauss-Bonnet gravity. As a by-product, we obtain the boundary entropy and A-type boundary central charges in general dimensions. We also study AdS/BCFT for general curvature-squared gravity. We find that it is too restrictive for the shape of the brane and the dual BCFT is trivial if one imposes Neumann boundary conditions for all of the gravitational modes. Instead, we propose to impose Dirichlet boundary condition for the massive graviton, while imposing Neumann boundary condition for the massless graviton. In this way, we obtain non-trivial shape dependence of stress tensor and well-defined central charges. In particular, the holographic g-theorem is satisfied by general curvature-squared gravity. Finally, we discuss the island and show that the Page curve can be recovered for Gauss-Bonnet gravity. Interestingly, there are zeroth-order phase transitions for the Page curve within one range of couplings obeying causality constraints. Generalizing the discussions to holographic entanglement entropy and holographic complexity in AdS/CFT, we get new constraints for the Gauss-Bonnet coupling, which is stronger than the causality constraint.