论文标题

FCC金属中的断开连接介导的双胞胎/双结迁移

Disconnection-Mediated Twin/Twin-Junction Migration in FCC metals

论文作者

Xu, Mingjie, Chen, Kongtao, Cao, Fan, Estrada, Leonardo Velasco, Kaufman, Thomas M., Ye, Fan, Hahn, Horst, Han, Jian, Srolovitz, David J., Pan, Xiaoqing

论文摘要

我们介绍了新颖的,时间分辨的结果,原位HRTEM观察,分子动力学(MD)模拟和断开理论,这些理论阐明了通过与GB Triple-Triple-triple-contions(TJ)的隔离运动/反应,阐明了多晶材料中晶界运动(GBS)在多晶材料中的运动(GBS)的机制。我们专注于由一对相干双边界(CTB)和σ9GB组成的TJ。至于所有GB,断开理论意味着可以使用多种模式/局部机制进行CTB迁移,并且模式选择受迁移驱动力的性质的影响。尽管我们通过化学势跳跃驱动的纯步骤观察(HRTEM和MD)CTB迁移,但其他实验观察(和我们的模拟)表明,压力驱动的CTB迁移是通过与非零汉堡室矢量的脱节的运动来发生的。这些是纯步骤和孪生派对的CTB迁移机制。我们的实验观察结果和模拟表明,GB的运动拖动了其划界TJ,并可能迫使TJ其他GBS会议的运动。我们的实验和模拟集中在两种由CTB和σ9GB组成的TJ上。 107°TJ很容易迁移,而70°TJ则与我们的断开理论一致(实验,模拟),即使组成型GB的固有迁移率不取决于TJ型型。我们还证明,在TJ(化学势跳/应力驱动)和GB/游离表面连接处(应力驱动)上可能形成断开连接。

We present the results of novel, time-resolved, in situ HRTEM observations, molecular dynamics (MD) simulations, and disconnection theory that elucidate the mechanism by which the motion of grain boundaries (GBs) in polycrystalline materials are coupled through disconnection motion/reactions at/adjacent to GB triple junctions (TJs). We focus on TJs composed of a pair of coherent twin boundaries (CTBs) and a Σ9 GB. As for all GBs, disconnection theory implies that multiple modes/local mechanisms for CTB migration are possible and that the mode selection is affected by the nature of the driving force for migration. While we observe (HRTEM and MD) CTB migration through the motion of pure steps driven by chemical potential jump, other experimental observations (and our simulations) show that stress-driven CTB migration occurs through the motion of disconnections with a non-zero Burgers vector; these are pure-step and twinning-partial CTB migration mechanisms. Our experimental observations and simulations demonstrate that the motion of a GB drags its delimiting TJ and may force the motion of the other GBs meeting at the TJ. Our experiments and simulations focus on two types of TJs composed of a pair of CTBs and a Σ9 GB; a 107° TJ readily migrates while a 70° TJ is immobile (experiment, simulation) in agreement with our disconnection theory even though the intrinsic mobilities of the constituent GBs do not depend on TJ-type. We also demonstrate that disconnections may be formed at TJs (chemical potential jump/stress driven) and at GB/free surface junctions (stress-driven).

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