论文标题

旋转纳米颗粒的三维相干布拉格成像

Three-dimensional coherent Bragg imaging of rotating nanoparticles

论文作者

Björling, Alexander, Marçal, Lucas A. B., Solla-Gullón, José, Wallentin, Jesper, Carbone, Dina, Maia, Filipe R. N. C.

论文摘要

Bragg相干衍射成像(BCDI)是一种强大的应变成像工具,通常受到小颗粒和高功率密度的样品不稳定性的限制。在这里,我们设计并验证了适应的衍射体积组件算法,能够从未经控制和未知旋转的粒子中恢复三维数据集。我们将方法应用于在聚焦相干X射线梁的影响下旋转的金纳米颗粒,从而取回其三维形状和应变场。结果表明,可以克服样本不稳定性问题,从而使BCDI的第四代同步加速器源使用其全部潜力。

Bragg Coherent Diffraction Imaging (BCDI) is a powerful strain imaging tool, often limited by beam-induced sample instability for small particles and high power densities. Here, we devise and validate an adapted diffraction volume assembly algorithm, capable of recovering three-dimensional datasets from particles undergoing uncontrolled and unknown rotations. We apply the method to gold nanoparticles which rotate under the influence of a focused coherent X-ray beam, retrieving their three-dimensional shapes and strain fields. The results show that the sample instability problem can be overcome, enabling the use of fourth generation synchrotron sources for BCDI to their full potential.

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