论文标题

在SR $ _2 $ CRREO $ _6 $中,反相域边界之间的强大远程磁相关

Robust Long Range Magnetic Correlation across Anti-phase Domain Boundaries in Sr$_2$CrReO$_6$

论文作者

Yuan, Bo, Kim, Subin, Chun, Sae Hwan, Jin, Wentao, Nelson, C. S., Hauser, Adam J., Yang, F. Y., Kim, Young-June

论文摘要

抗位点疾病是合成双钙钛矿用于旋转器应用的最重要问题之一。尽管众所周知,抗部位疾病会导致结构缺陷的增殖,即样品中分离有序的反相结构域分离有序的反相结构域的反相边界,但对于微观水平上这些反相边界的磁相关知识知之甚少。在此激励的情况下,我们报告了在SR $ _2 $ _2 $ crreo $ _6 $的薄膜样本中室温磁性和结构相关性的共振弹性X射线散射研究,该样本在双perovskites中具有最高的$ \ mathrm {t_c} $之一。从结构上讲,我们发现了样本中$ \ sim $ 15〜nm的抗相纳米域的存在。从磁性上讲,订购的矩显示出垂直于$ c $方向的位置。最值得注意的是,我们发现磁相关长度远远超过了单个抗相纳米构域的大小。因此,我们的结果为在SR $ _2 $ crreo $ _6 $中的反相边界上存在强大的磁相关性提供了结论性的证明。

Anti-site disorder is one of the most important issues that arises in synthesis of double perovskite for spintronic applications. Although it is known that anti-site disorder leads to a proliferation of structural defects, known as the anti-phase boundaries that separate ordered anti-phase domains in the sample, little is known about the magnetic correlation across these anti-phase boundaries on a microscopic level. Motivated by this, we report resonant elastic X-ray scattering study of room temperature magnetic and structural correlation in a thin-film sample of Sr$_2$CrReO$_6$, which has one of the highest $\mathrm{T_C}$ among double perovskites. Structurally, we discovered existence of anti-phase nanodomains of $\sim$15~nm in the sample. Magnetically, the ordered moments are shown to lie perpendicular to the $c$ direction. Most remarkably, we found that the magnetic correlation length far exceeds the size of individual anti-phase nanodomains. Our results therefore provide conclusive proof for existence of robust magnetic correlation across the anti-phase boundaries in Sr$_2$CrReO$_6$.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源