论文标题

大区域CVD石墨烯中声学等离子体的真实空间成像

Real-space imaging of acoustic plasmons in large-area CVD graphene

论文作者

Menabde, Sergey G., Lee, In-Ho, Lee, Sanghyub, Ha, Heonhak, Heiden, Jacob T., Yoo, Daehan, Kim, Teun-Teun, Lee, Young Hee, Low, Tony, Oh, Sang-Hyun, Jang, Min Seok

论文摘要

在石墨烯 - 二电 - 基准异质结构中,一种声学等离子体模式最近被视为强烈的光 - 物质相互作用的卓越平台。它源自石墨烯等离子体与镜像图像的耦合,并在Nm厚度介电的极限上表现出最大的场限制。尽管最近在远场状态中检测到,但该模式的光学近场尚未观察到和表征。石墨烯边缘通过近场散射显微镜反射的等离子场的直接光学探测显示,我们设备中MID-IR声学等离子的阻尼速率相对较小,即使在环境条件下,即使在未受保护的,化学上生长的大区域的大区块的大区块也可以进行实际空间映射。我们显示的声学模式是限制的两倍,但在相似条件下的石墨烯表面等离子体上,减湿的1.4倍。我们还以1D阵列的金纳米管阵列对远场耦合的高效率进行成像。我们的结果强调了声学等离子体作为在MID-IR中运行的大面积石墨烯的光电设备的异常有希望的平台的重要性。

An acoustic plasmonic mode in a graphene-dielectric-metal heterostructure has recently been spotlighted as a superior platform for strong light-matter interaction. It originates from the coupling of graphene plasmon with its mirror image and exhibits the largest field confinement in the limit of a nm-thick dielectric. Although recently detected in the far-field regime, optical near-fields of this mode are yet to be observed and characterized. Direct optical probing of the plasmonic fields reflected by the edges of graphene via near-field scattering microscope reveals a relatively small damping rate of the mid-IR acoustic plasmons in our devices, which allows for their real-space mapping even with unprotected, chemically grown, large-area graphene at ambient conditions. We show an acoustic mode that is twice as confined - yet 1.4 times less damped - compared to the graphene surface plasmon under similar conditions. We also image the resonant acoustic Bloch state in a 1D array of gold nanoribbons responsible for the high efficiency of the far-field coupling. Our results highlight the importance of acoustic plasmons as an exceptionally promising platform for large-area graphene-based optoelectronic devices operating in mid-IR.

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