论文标题
活性手性颗粒的动力学结晶石
Dynamical Crystallites of Active Chiral Particles
论文作者
论文摘要
远程平衡系统的内在特征之一是系统动力学的非递归性质,它导致新的特性,这些特性无法理解和通过基于热力学潜能的常规途径来理解和描述。特别感兴趣的是由表现出集体行为的有效粒子组成的有序模式的形成和演变。在这里,我们研究了这种非电势活动系统,重点是耦合和手性粒子自我启动与自旋之间的竞争的影响。它导致了由集体翻译运动,旋转引起的结构停滞和动态挫败感主导的三个散装动力学方案之间的过渡。此外,由于由晶体熔体界面引起的局部偏置过渡,持续的自动旋转晶体的动态状态被确定。也可以利用破坏局部散装状态的机制来实现主动晶体层的自发或自流。
One of the intrinsic characteristics of far-from-equilibrium systems is the nonrelaxational nature of the system dynamics, which leads to novel properties that cannot be understood and described by conventional pathways based on thermodynamic potentials. Of particular interest are the formation and evolution of ordered patterns composed of active particles that exhibit collective behavior. Here we examine such a type of nonpotential active system, focusing on effects of coupling and competition between chiral particle self-propulsion and self-spinning. It leads to the transition between three bulk dynamical regimes dominated by collective translative motion, spinning-induced structural arrest, and dynamical frustration. In addition, a persistently dynamical state of self-rotating crystallites is identified as a result of a localized-delocalized transition induced by the crystal-melt interface. The mechanism for the breaking of localized bulk states can also be utilized to achieve self-shearing or self-flow of active crystalline layers.