论文标题
用拓扑结构手性液滴调整微叠剂的手性
Tailoring the Chirality of Microlaser with Topological Structured Chiral Droplets
论文作者
论文摘要
手性激光发射的产生为现代光子应用和手性光伴侣相互作用提供了有希望的机会。尽管近年来做出了巨大的过程,但具有可控手性的直接生成手性激光在微腔中仍然具有挑战性。这项研究报告了一种控制拓扑结构的手性液晶液滴的窃窃私语模式有机微叠剂的发射手性的策略。研究结果表明,微螺旋体中的拓扑转换可以诱导不同的光学手性强度和激光极化特征。特别是,在线性和圆形极化激发下还研究了光旋转功率的作用,在线和圆极化激励下,揭示了左/右圆极化激发之间的巨大激光强度差。进行理论分析和模拟以支持重要的发现。这项研究提供了一种轻松的工具,用于操纵微腔中的手性激光排放,从而为拓扑控制的光子学,手性光学设备和手性分子检测提供了灵感。
The generation of chiral laser emission offers promising opportunities for modern photonic applications and the study of chiral light-mater interactions. Despite the great process made in recent years, the direct generation of chiral lasers with controllable chirality remains challenging in a microcavity. This study reports a strategy to control the emission chirality of whispering-gallery-mode organic microlasers with topological-structured chiral liquid crystal droplets. The findings suggest that the topological transformations in a microdroplet can induce different optical chirality strength and lasing polarization characteristics. In particular, the role of optical rotatory power was also investigated under linear and circular polarized excitation, where a vast lasing intensity difference between left/right circular polarized excitation was revealed. Theoretical analysis and simulation were carried out to support the significant findings. This study provides a facile tool for manipulating chiral laser emissions in microcavity, giving inspiration for topological-controlled photonics, chiral optical devices, and chiral molecular detection.