论文标题

带有分离的Ru3O12-Trimer的BA5RU3O12中的复杂磁结构

Complex magnetic structure in Ba5Ru3O12 with isolated Ru3O12-trimer

论文作者

Basu, T., Wei, F. Y., Zhang, Q., Fang, Y., Ke, X.

论文摘要

我们报告了BA5RU3O12的详细磁性,传输,热容量和中子衍射测量,该测量由隔离的RU3O12夹子组成。我们表明,该系统在60 K(TN)下开发了远程抗磁磁有序,而没有结构变形和金属隔离剂型跃迁,这与其他氟丁酸三聚体系统(如9R-Baruo3和Ba4ru3O10)形成了鲜明的对比。揭示了一个复杂的磁性结构,这归因于RU3O12夹子内不同晶体学位点上RU离子之间的竞争交换相互作用引起的磁性挫败感。

We report detailed magnetic, transport, heat-capacity, and neutron diffraction measurements of Ba5Ru3O12, a compound consisting of isolated Ru3O12 trimers. We show that this system develops long-range antiferromagnetic ordering at 60 K (TN) without structural distortion and metal-insulator-type transition, which is in sharp contrast to other Barium Ruthenate trimer systems such as 9R-BaRuO3 and Ba4Ru3O10. A complex magnetic structure is revealed which is attributable to the magnetic frustration due to competing exchange interactions between Ru ions on different crystallographic sites within the Ru3O12 trimer.

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