论文标题
稀释YB中磁化二聚体的实验性观察:Yalo $ _3 $
Experimental observation of magnetic dimers in diluted Yb:YAlO$_3$
论文作者
论文摘要
我们对Yb $ _ {0.04} $ y $ _ {0.96} $ alo $ _3 $的Yb磁化液进行了全面的实验研究,一个YB掺杂的Yttrium yttrium aluminum perovskite(yap)yalo $ _3 $ yalo $ _3 $,通过特定的热量,磁性化,磁性量和高量度分散(深度均匀的中性均匀分散)。在我们的样本中,YB离子是随机分布在晶格上的,$ \ sim 7 $ \%yb离子形式量子二聚体,由于最近邻居抗铁磁耦合沿$ c $轴轴。在零字段,二聚体的形成在INS频谱中的非弹性峰的外观大约为0.2 $ 〜MEV,并且在特定热量中表现出schottky样异常。 INS峰的结构因子沿$ L $方向展示了余弦调制,与$ c $轴接近邻居内二聚体耦合一致。仔细拟合低温特异性热的热量表明,激发态是一个退化的三胞胎,这表明尽管晶体对称性低和各向异性磁性偶极贡献,但有效的YB-YB交换相互作用的各向异性与先前的报道一致,Yb parent yb parent $ _3 $ _3 $ _112:1903.1133.11333.113 3.113 3.113 3.113 3.1133.1133.1133.1133.11333。arcy and and and and yb yb-yb交换相互作用。与yb $ _2 $ pt $ _2 $ pb [arxiv:1606.01309,arxiv:1907.01067]形成鲜明对比。获得的结果通过YB二聚体的分析计算精确地再现。
We present a comprehensive experimental investigation of Yb magnetic dimers in Yb$_{0.04}$Y$_{0.96}$AlO$_3$, an Yb-doped Yttrium Aluminum Perovskite (YAP) YAlO$_3$ by means of specific heat, magnetization and high-resolution inelastic neutron scattering (INS) measurements. In our sample, the Yb ions are randomly distributed over the lattice and $\sim 7$\% of Yb ions form quantum dimers due to nearest-neighbor antiferromagnetic coupling along the $c$-axis. At zero field, the dimer formation manifests itself in an appearance of an inelastic peak at $Δ\approx 0.2$~meV in the INS spectrum and a Schottky-like anomaly in the specific heat. The structure factor of the INS peak exhibits a cosine modulation along the $L$ direction, in agreement with the $c$-axis nearest-neighbor intra-dimer coupling. A careful fitting of the low-temperature specific heat shows that the excited state is a degenerate triplet, which indicates a surprisingly small anisotropy of the effective Yb-Yb exchange interaction despite the low crystal symmetry and anisotropic magnetic dipole contribution, in agreement with previous reports for the Yb parent compound, YbAlO$_3$ [arXiv:1904.11513, arXiv:1902.04112], and in contrast to Yb$_2$Pt$_2$Pb [arXiv:1606.01309, arXiv:1907.01067]. The obtained results are precisely reproduced by analytical calculations for the Yb dimers.