论文标题

van der waals 1T-VSE $ _2 $层的相干生长和表征使用分子束外延(111)b(111)b

Coherent Growth and Characterization of van der Waals 1T-VSe$_2$ Layers on GaAs(111)B Using Molecular Beam Epitaxy

论文作者

Zhu, Tiancong, O'Hara, Dante J., Noesges, Brenton A., Zhu, Menglin, Repicky, Jacob J., Brenner, Mark R., Brillson, Leonard J., Hwang, Jinwoo, Gupta, Jay A., Kawakami, Roland K.

论文摘要

我们报告了通过分子束外观上的八面体配位(1T)结构中二叶发展式(1T)结构中菜籽硅胶(VSE $ _2 $)薄膜的外延生长。显示了最高30 mL的单个单层(ML)的膜厚度。使用X射线衍射,透射电子显微镜,扫描隧道显微镜和X射线光电子光谱的结构和化学研究表明高质量的薄膜。进一步的研究表明,GAAS上的单层VSE $ _2 $胶片不是空气稳定的,并且在几个小时内容易受到氧化的影响,这表明应将保护性封盖层用于设备应用。这项工作表明,可以通过2D/3D混合设备的外延生长将VSE $ _2 $(用于可能的Spintronic和电子应用的候选范德华材料)与III-V半导体集成。

We report epitaxial growth of vanadium diselenide (VSe$_2$) thin films in the octahedrally-coordinated (1T) structure on GaAs(111)B substrates by molecular beam epitaxy. Film thickness from a single monolayer (ML) up to 30 ML is demonstrated. Structural and chemical studies using by x-ray diffraction, transmission electron microscopy, scanning tunneling microscopy and x-ray photoelectron spectroscopy indicate high quality thin films. Further studies show that monolayer VSe$_2$ films on GaAs are not air-stable and are susceptible to oxidation within a matter of hours, which indicates that a protective capping layer should be employed for device applications. This work demonstrates that VSe$_2$, a candidate van der Waals material for possible spintronic and electronic applications, can be integrated with III-V semiconductors via epitaxial growth for 2D/3D hybrid devices.

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