论文标题

通过扩展的近藤效应揭示单个磁分子内的原子位点依赖性g因子

Revealing the Atomic Site-Dependent g Factor within a Single Magnetic Molecule via the Extended Kondo Effect

论文作者

Liu, Liwei, Yang, Kai, Jiang, Yuhang, Song, Boqun, Xiao, Wende, Song, Shiru, Du, Shixuan, Ouyang, Min, Hofer, Werner A., Neto, Antonio H. Castro, Gao, Hong-Jun

论文摘要

单个磁分子的位点依赖性g因子具有分子内分辨率,首次通过低温,高磁场的高磁场扫描隧穿显微镜在AU上的脱氢Mn-苯羟苯胺分子的隧道显微镜证明(111)。这是通过探索分子不同原子位点的扩展近代效应的磁场依赖性来实现的。重要的是,揭示了单个分子内G因子的不均匀分布。我们的结果开辟了一条新的途径,以访问单个分子中的局部自旋特性。

The site-dependent g factor of a single magnetic molecule, with intramolecular resolution, is demonstrated for the first time by low-temperature, high-magnetic-field scanning tunneling microscopy of dehydrogenated Mn-phthalocyanine molecules on Au(111). This is achieved by exploring the magneticfield dependence of the extended Kondo effect at different atomic sites of the molecule. Importantly, an inhomogeneous distribution of the g factor inside a single molecule is revealed. Our results open up a new route to access local spin properties within a single molecule.

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