论文标题
透视图:[111]生长金属氧化物薄膜和异质结构的密切相关和拓扑状态
Perspective: Strongly correlated and topological states in [111] grown transition metal oxide thin films and heterostructures
论文作者
论文摘要
我们重点介绍了[111]面向过渡金属氧化物薄膜和异质结构中强相关性和拓扑状态的理论,材料制造以及实验表征的最新进展,与其[001]方向的对应物相比,这是难以实现的。我们专注于两类复杂的氧化物,包括化学配方ABO3和A2B2O7,其中B位点被带有局部时刻的开放壳过渡金属离子占据,而A位点通常是稀土。 [111]源自这些母体化合物晶格的定向的准二维晶格可以表现出特殊的几何形状和对称性,即弯曲的蜂窝状晶格,以及kagome和kagome和三角形lattices。这些晶格图案构成了以异国情调的磁性,各种形式的轨道秩序,拓扑绝缘子,拓扑半学,量子异常的霍尔绝缘子和量子旋转液体表达的紧密相关和拓扑状态的基础。对于具有较高原子数的过渡金属离子,自旋轨道耦合起着重要作用,并可能在电子带结构和磁激发频谱中产生其他拓扑特征。我们通过在这个积极发展的领域中阐明公开挑战和机遇来结束观点。
We highlight recent advances in the theory, materials fabrication, and experimental characterization of strongly correlated and topological states in [111] oriented transition metal oxide thin films and heterostructures, which are notoriously difficult to realize compared to their [001] oriented counterparts. We focus on two classes of complex oxides, with the chemical formula ABO3 and A2B2O7, where the B sites are occupied by an open-shell transition metal ion with a local moment, and the A sites are typically a rare earth. The [111] oriented quasi-two-dimensional lattices derived from these parent compound lattices can exhibit peculiar geometries and symmetries, namely, a buckled honeycomb lattice, as well as kagome and triangular lattices. These lattice motifs form the basis for emergent strongly correlated and topological states expressed in exotic magnetism, various forms of orbital ordering, topological insulators, topological semimetals, quantum anomalous Hall insulators, and quantum spin liquids. For transition metal ions with high atomic number, spin-orbit coupling plays a significant role and may give rise to additional topological features in the electronic band structure and in the spectrum of magnetic excitations. We conclude the Perspective by articulating open challenges and opportunities in this actively developing field.