论文标题

牙脲硫化葡萄糖剂Zn1-Xcuxir2-yn(n = al,ti,rh)yte4的电荷密度波和超导性

Charge density wave and superconductivity in the family of telluride chalcogenides Zn1-xCuxIr2-yN(N = Al, Ti, Rh)yTe4

论文作者

Yan, Dong, Zeng, Yijie, Lin, Yishi, Zeng, Lingyong, Yin, Junjie, He, Yuan, Boubeche, Mebrouka, Wang, Meng, Wang, Yihua, Yao, Dao-Xin, Luo, Huixia

论文摘要

超导性和电荷密度波(CDW)/金属对绝缘体过渡(MIT)之间的相互作用长期以来一直在凝结物理学中一直感兴趣并研究。在这里,我们系统地研究固体溶液Zn1-XCUXIR2-YN(n = al,Ti,rh)YTE4中的电荷密度波和超导性能。电阻率,磁化率和特定的热量测量表明,CDW状态立即被抑制,而超导临界温度(TC)与每个系统有所不同。在AL和TI实施案例中,TC随着Y的增加而增加,在Y = 0.075时分别达到2.75 K和2.84 K左右,然后在Y = 0.2达到化学相边界之前的TC降低。然而,随着RH掺杂含量Y的增加,TC单调减小,并在0.3以上消失,测量温度降低至2K。令人惊讶的是,在Zn1-XCUXIR2TE4固定溶液中,TC随着X = 0.5的最大范围而在0.5的范围内较高,TC随着X = 0.5的范围而增强,TC随着X的最大值而达到2.82 K的最大值,而DC的范围为0.9,则X型较大的范围较大,而DC的范围较高。观察锌掺杂的观察会迅速抑制高TC Cuprate超导体中的超导性。代表性最佳掺杂样品的超导转变处的特定热异常均略高于1.43的BCS值,并指示这些化合物中的大量超导性。最后,已经建立并进行了比较,与Zn1-XCUXIR2-YN(N = AL,TI,RH)YTE4的CDW过渡温度(TCDW)和超导转换温度(TC)与X/Y含量相图相比,这为研究CDW和超级传导性之间的竞争提供了很好的机会。

The interplay between superconductivity and charge density wave (CDW)/metal-to-insulator transition (MIT) has long been interested and studied in condensed matter physics. Here we study systematically the charge density wave and superconductivity properties in the solid solutions Zn1-xCuxIr2-yN(N = Al, Ti, Rh)yTe4. Resistivity, magnetic susceptibility and specific heat measurements indicate that the CDW state was suppressed immediately while the superconducting critical temperature (Tc) differs from each system. In the Al- and Ti-substitution cases, Tc increase as y increases and reaches a maximum around 2.75 K and 2.84 K respectively at y = 0.075, followed by a decrease of Tc before the chemical phase boundary is reached at y = 0.2. Nevertheless, Tc decreases monotonously with Rh-doping content y increases and disappears above 0.3 with measuring temperature down to 2 K. Surprisingly, in the Zn1-xCuxIr2Te4 solid solution, Tc enhances as x increases and reaches a maximum value of 2.82 K for x = 0.5 but subsequently survives over the whole doping range of 0.00 - 0.9 despite Tc changes slightly with higher doping content, which differs from the observation of zinc doping suppressing the superconductivity quickly in the high Tc cuprate superconductors. The specific heat anomaly at the superconducting transitions for the representative optimal doping samples are all slightly higher than the BCS value of 1.43 and indicate bulk superconductivity in these compounds. Finally, the CDW transition temperature (TCDW) and superconducting transition temperature (Tc) vs. x/y content phase diagrams of Zn1-xCuxIr2-yN(N = Al, Ti, Rh)yTe4 have been established and compared, which offers good opportunity to study the competition between CDW and superconductivity in the telluride chalcogenides.

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