论文标题

三角晶格tlybs $ _2 $ crystals在熔融通量中生长

Frustrated Magnetism in Triangular Lattice TlYbS$_2$ Crystals Grown via Molten Flux

论文作者

Ferreira, Timothy, Xing, Jie, Sanjeewa, Liurukara D., Sefat, Athena S.

论文摘要

三角形晶格化合物Tlybs $ _2 $是通过使用氯化钠的熔融通量生长技术作为大型单晶制备的。至0.4 K的各向异性磁敏感性测量表明完全没有远程磁性。尽管缺乏远距离的顺序,但通过广泛的过渡证明了短距离抗铁磁相互作用,这表明行为沮丧。可变的磁场测量结果显示在小于2 K的温度下的元磁行为。复杂的低温场可感应磁性行为,除了没有可观察到的长距离顺序降至0.4 K,这表明Tlybs $ _2 $是沮丧的磁铁和可能的量子量旋转液体候选者。

The triangular lattice compound TlYbS$_2$ was prepared as large single crystals via a molten flux growth technique using sodium chloride. Anisotropic magnetic susceptibility measurements down to 0.4 K indicate a complete absence of long-range magnetic order. Despite this lack of long-range order, short-range antiferromagnetic interactions are evidenced through broad transitions, suggesting frustrated behavior. Variable magnetic field measurements reveal metamagnetic behavior at temperatures less than 2 K. Complex low temperature field-tunable magnetic behavior, in addition to no observable long-range order down to 0.4 K, suggest that TlYbS$_2$ is a frustrated magnet and a possible quantum spin liquid candidate.

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